nukwastpats


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**Nuclear Waste Remediation/Transmutation**

**Patents**

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 **USP Application 2002169351** **Remediation of Radioactive Waste by Stimulated
Radioactive Decay** 


**Paul M.
Brown**

Disclosed is a radioactive waste treatment
process for transmuting long-lived radioisotopes into
short-lived radioisotopes through applied nuclear physics.
Nuclear reactions, specifically of the (gamma, n) type, also
known as photodisintegration, are utilized to accomplish
this transmutation from troublesome, long-lived radioactive
waste isotope(s) of given atomic mass to shorter-lived or
stable materials of lower atomic mass, by exposing the
troublesome isotopes to a high energy photon flux for a
sustained time. Generally speaking, the target nucleus of
the radioisotope(s) to be treated is irradiated by gamma
photons of an energy greater than the binding energy of the
neutron in the target nucleus. This causes the irradiated
nucleus to absorb the gamma rays, thereby placing the
nucleus in an excited state. Upon relaxation, the nucleus
ejects a neutron through the (gamma, n) reaction, thereby
transmuting the element to an isotope of lower atomic mass
and shorter half-life  
.

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**WO
Patent # 9,403,906**

**Methods for Manufacturing & Producing
Products**

 

**Ronald
Brightsen, et al.**

A method for generating high energy 32He particles includes
the steps of accumulating protons and deuterons in intimate
contact with a lattice structure storage member and
repeatedly reacting one proton and one deuteron to produce
32He particles and excess energy greater than 6 MeV for each
of the 32He particles. A method for controlling an energy
production reaction of isotopic hydrogen atoms includes
steps for storing a first isotope of hydrogen and a second
isotope of hydrogen in contact with a lattice structure to
produce a first ratio of the first isotope to the second
from a mixture having a second ratio of the first isotope to
the second isotope, adjusting the energy of the lattice
structure to initiate the energy production reaction caused
by the interaction of one nucleus of the first isotope with
one nucleus of the second isotope and controlling the second
ratio to control the rate of the energy production reaction
based on the interaction of the first isotope with the
second isotope. Methods for treating radioactive waste by
transmutation and for forming a superconductive material
from a plurality of constituents, as well as methods for
forming improved semiconductor devices, improved atomic
lattice structures and improved molecular structures and
ionic compounds, are described along with selection rules
for fine tuning these methods. An apparatus for producing
controlled emissions of high energy vHe particles, which can
be adapted as a beam producing device or as motor, is also
disclosed.

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**WO03098640**  
 **Processing Radioactive
Materials with Hydrogen Isotope Nuclei**

**John Dash**

Embodiments of a method for processing
radioacive materials, with a particular embodiment
comprising processing uranium with hydrogen isotope plasmas,
and a process for remediation of nuclear wastes by
transmutation.

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**DE19803629**  
 **Transmutation of Isotopes
with Long Half Life**

 

**Heinrich
Hora**

For the transmutation of long half-life
isotopes, their surfaces are exposed to an electrolyte or a
gas or plasma atmosphere to form intermediate layers or vol.
zones of a number of structure layers. The threshold zones
are placed against a carrier material or close to vol. zones
of metals or metal layers, composed of metals capable of
absorbing \-1 atom% of hydrogen or its isotope.

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**Japan
Patent 9197077**  
 **Electrode for Cold Nuclear
Fusion & Method for Manufacturing
Radioactive & Nonradioactive Element &
Pervious Metal by Nuclear Transformation in
Electrode**

 

**Reiko
Notoya**

To obtain an electrode for cold nuclear fusion
which can manufacture isotopes, precious metals, rare
elements or thermal energy through nuclear transformation by
containing as a material for the electrode a substance which
can cause nuclear transformation. Solution: Radioactive or
nonradioactive isotopes are manufactured by the nuclear
transformation in an electrode and the combination of
nuclear reactions such as neutron capture and natural
nuclear disintegration of products made through the nuclear
reactions. The kinds of manufactured isotopes are very
numerous, and it is especially easy to obtain non-single
isotopes. Since the conditions of electrolysis can be
controlled very precisely, it is possible to manufacture
only target substances precisely. For an electrode for cold
nuclear fusion, an element whose atomic number is close to
that of a precious metal or a rare element is chosen as a
substance which can cause nuclear transformation, or a
material for the nuclear transformation of a precious metal
and a rare element. For example, W, Ag, Sn and Pt are cited
as materials for platinum-family metals and gold. As
materials for rare elements, chemical species such as the
halogen family, alkaline metals, Po and W are chosen.

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**US6738446**   
**System and method for radioactive waste
destruction**  
  
**Venneri, et al.**  
  
A method for transmuting spent fuel from a nuclear reactor
includes the step of separating the waste into components
including a driver fuel component and a transmutation fuel
component. The driver fuel, which includes fissile materials
such as Plutonium.sup.239, is used to initiate a critical,
fission reaction in a reactor. The transmutation fuel, which
includes non-fissile transuranic isotopes, is transmuted by
thermal neutrons generated during fission of the driver
fuel. The system is designed to promote fission of the
driver fuel and reduce neutron capture by the driver fuel.
Reacted driver fuel is separated into transuranics and
fission products using a dry cleanup process and the
resulting transuranics are mixed with transmutation fuel and
re-introduced into the reactor. Transmutation fuel from the
reactor is introduced into a second reactor for further
transmutation by neutrons generated using a proton beam and
spallation target.

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**RU2052223**   
**Method For Producing Stable Isotopes Due To
Nuclear Transmutation, Such As Low-Temperature Nuclear
Fusion Of Elements In Microbiological
Cultures**  
  
**V. Vysotskij / A. Kornilova**  
  
A method of obtaining stable isotopes by nuclear fusion of
elements in microbial cultures, including the preparation of
the culture medium for the growth of microbiological
cultures deficient isotope obtainable by transmutation, and
containing the necessary transmutation initial isotopic
components; growing in a nutrient medium microbiological
cultures requiring these isotopes for their growth,
isolating from the culture medium grown culture and
isolation of stable isotopes [2] In the conventional method
describes the procedure for growing microbiological cultures
Aspergillus niger IFO 4066, Penicillium chrysogenum IFO
4689; Phizopus nigricans IFO 5781; Mucor rouxii IFO 0369;
Saccharomuces cerevisiae IFO 0308 ; Torulopsis utilis IFO
0396; Saccharomyces ellipideus IFO 0213; Hansenula anomala
IFO 0118 in a nutrient medium is an aqueous solution of a
number of chemical compounds and deficient in one of the
essential components for the growth of crops (potassium,
magnesium, iron, calcium) and for monitoring, standard for
them spedi. In experiments on the implementation of the
method has been shown that the cultivation of these crops in
the corresponding element deficient media (data media in
these specific elements did not exist) in the resulting
culture of these elements were present, which can only be
attributed to their synthesis in the nuclear transmutation
of the other elements present, and isotopes.

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**RU2034414**  
**Accelerating Complex For Transmutation Of
Nuclear Production Waste**   
  
**M. Danilov / Y. Katarzhnov**

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**GB2246467**  
**Transmutation treatment of radioactive
wastes**  
  
**K. Konashi / N. Sasao**  
  
A method for the transmutation treatment of
radioactive wastes comprises: accelerating radioactive
nuclides contained in the radioactive wastes to be treated
to an energy level corresponding to a compound nucleus
resonance level; and bombarding the accelerated nuclides
into a thermal neutron field, which is under a magnetic
field, to cause the compound nucleus resonance reaction to
occur; thereby transforming the radioactive nuclides into
those which are more stable or have shorter life. The
nuclides are accelerated in accelerator 9 then passed into
an annular-cylindrical chamber 3 positioned about a reactor
1 where they are treated with neutrons.

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**US4721596**  
**Method for net decrease of hazardous radioactive
nuclear waste
materials**  
  
**R. Marriott / F. Henyey**  
  
A method for decreasing the amount of hazardous radioactive
reactor waste materials by separation from the waste of
materials having long-term risk potential and exposing these
materials to a thermal neutron flux. The utilization of
thermal neutrons enhances the natural decay rates of the
hazardous materials while the separation for recycling of
the hazardous materials prevents further transmutation of
stable and short-lived nuclides.

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**EP0030404**  
**Method for net decrease of hazardous radioactive
nuclear waste
materials.**  
  
**R. Marriott / F. Henyey**  
  
Also published as: ZA8007201 / JPS56125698 / AU6435380 /
AU539393  
  
A method for decreasing the amount of hazardous radioactive
reactor waste materials by separating from the waste of
materials having long-term risk potential and exposing these
materials to a thermal neutron flux. The utilization of
thermal neutrons enhances the natural decay rates of the
hazardous materials while the separation for recycling of
the hazardous materials prevents further transmutation of
stable and short-lived nuclides.

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**GB970091**  
**Transmutation of
elements**  
  
**I. Noel**  
  
Transmutation of elements. N. I. RAFFERTY. Sept. 10,1963
[June 19,1962], No. 23586/62. Heading G6P. A process for the
synthesis of helium and the simultaneous generation of
energy comprises admixing in a steel pressure-tight vessel
in presence of air following reactants in the following
order: aluminium in a physical form presenting a large
volume/surface ratio, solid sodium hydroxide, and water in
the ratio of 4 : 8 : 8. The reaction is stated to be
thermonuclear involving the carbon cycle proposed by Bethe,
the effect of which is to transmute hydrogen into helium

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**JP2004117106**  
**Structure For Nuclide Transmutation And Method
For Forming It**  
  
**T. Ito Takehiko / M. Sakano**  
  
To provide a structure for transmuting nuclides with a
relatively small-scale device and a means for manufacturing
the structure. ; SOLUTION: A mixed layer consisting of
lamination layers of a Pd layer and a layer of a substance
which has a smaller work function than Pd is placed on a
substrate made of Pd, a Pd alloy, other metals occluding
hydrogen or alloys of these metals, the structure shaped
like an approximate plate where an additional Pd layer is
placed on the mixed layer is formed and a substance which is
given nuclide transmutation is supplied to the Pd layer of
the structure. The substance which is supplied to the Pd
layer and is given nuclide transmutation is acceptable if it
has become metallic, and salt may adhere to the surface of
it. Electrodeposition and ion implantation can be used as a
means for supplying the substance which is given nuclide
transmutation

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**FR2855309**  
**Plasma-free nucleon transmutation comprises use
of piezoelectric actuators to produce energy particles
compatible with targets**  
  
**G. Vitrac**  
    
Nucleon transmutation, initiated by plasma-free fusion uses
piezo-electric actuators to ensure particle transfer where
the velocity vector benefits from additional quantum that
favors collisions and automatically-triggered fusion. This
accords, in particular, with the laws of velocity
distribution and the probability of collisions for energy
particles compatible with targets.

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**US2003210759**  
**Nuclide transmutation device and nuclide
transmutation
method**  
  
**Y. Iwamura / T. Itoh**  
    
The present invention produces nuclide transmutation using a
relatively small-scale device. The device 10 that produces
nuclide transmutation comprises a structure body 11 that is
substantially plate shaped and made of palladium (Pd) or
palladium alloy, or another metal that absorbs hydrogen (for
example, Ti) or an alloy thereof, and a material 14 that
undergoes nuclide transmutation laminated on one surface 11A
among the two surfaces of this structure body 11. The one
surface 11A side of the structure body 11, for example, is
made a region in which the pressure of the deuterium is high
due to pressure or electrolysis and the like, and the other
surface 11B side, for example, is a region in which the
pressure of the deuterium is low due to vacuum exhausting
and the like, and thereby, a flow of deuterium in the
structure body 11 is produced, and nuclide transmutation is
carried out by a reaction between the deuterium and the
material 14 that undergoes nuclide transmutation.

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**RU2210630**  
**Facility For Generation Of Gas Mixture And
Transmutation Of Nuclei Of Atoms Of Chemical
Elements**   
  
**F. Kanarev / V.  Podobedov**  
  
Facility for generation of gas mixture and transmutation of
nuclei of atoms of chemical elements has body made of
dielectric material with though hole, interelectrode
chamber, cooling chamber for vapor condensation, vessel for
working solution, branch pipes to feed and drain working
solution, anode connected to positive pole of power supply
source and cathode connected to negative pole of power
supply source. Body has upper boss with internal cavity.
Cathode is brought into cathode space from above through
axial hole of upper boss. Internal space of boss
communicates with cooling chamber which space is connected
to vessel for working solution. EFFECT: simultaneous
generation of gas mixture and transmutation of nuclei of
atoms of chemical elements.

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**US6233298**  
**Apparatus for transmutation of nuclear reactor
waste**  
  
**Charles Bowman**  
  
A subcritical reactor-like apparatus for treating nuclear
wastes, the apparatus comprising a vessel having a shell and
an internal volume, the internal volume housing graphite.
The apparatus having means for introducing a fluid medium
comprising molten salts and plutonium and minor actinide
waste and/or fission products. The apparatus also having
means for introducing neutrons into the internal volume
wherein absorption of the neutrons after thermalization
forms a processed fluid medium through fission chain events
averaging approximately 10 fission events to approximately
100 fission events. The apparatus having additional means
for removing the processed fluid medium from the internal
volume. The processed fluid medium typically has no
usefulness for production of nuclear weapons.

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**US6233299**  
**Assembly for transmutation of a long-lived
radioactive
material**  
  
**T. Wakabayashi**  
  
A new transmutation assembly permits an efficient
transmutation of a long-lived radioactive material
(long-lived FP nuclides such as technetium-99 or iodine-129)
which was produced in the nuclear reactor. Wire-type members
of a long-lived radioactive material comprised of metals,
alloys or compounds including long-lived FP nuclides are
surrounded by a moderator material and installed in cladding
tubes to form FP pins. The FP pins, and nothing else, are
housed in a wrapper tube to form a transmutation assembly.
The wire-type members can be replaced by thin ring-type
members. The transmutation assemblies can be selectively and
at least partly loaded into a core region, a blanket region
or a shield region of a reactor core in a fast reactor. From
a viewpoint of reducing the influence on the reactor core
characteristics, it is optimal to load the transmutation
assemblies into the blanket region.

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**WO9919881**  
**Low Temperature Electrolytic Nuclear
Transmutation**   
  
**James Patterson / George Miley**  
  
A method for producing low temperature nuclear
transmutations by electrolysis in an aqueous media. New
elements produced by transmutation are identified as having
discrete peaks in occurrence by atomic number (Z) and by
atomic mass (A). New complex nuclei produced by
transmutation are idendified as having existed based upon
the nature and occurrences of fission transmutation elements
produced. The electrolytic cell (12) includes a
non-conductive housing (14) having an inlet (54) and an
outlet (56) and spaced apart first and second conductive
grids (38 & 44) positioned therein. A plurality of
cross-linked polymer non-metallic cores each having a
uniform conductive exterior metallic surface formed of a
high hydrogen absorbing material form a bed (35) of
conductive beads (36) closely packed within the housing (14)
in electrical contact with the first grid (38) adjacent the
inlet (54). An electric power source (15, 16) in the system
(10) is operably connected across the first and second grids

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**WO9740211**  
**System, Electrolytic Cell And Method For
Producing Excess Heat And For Transmutation By
Electrolysis**  
  
**James Patterson / George Miley**  
   
An electrolytic cell (12), system (10) and method for
producing excess quantities of heat as a result of low
temperature nuclear transmutations which occur during
electrolysis in an aqueous media within the cell (12). The
electrolytic cell (12) includes a non-conductive housing
(14) having an inlet (54) and an outlet (56) and spaced
apart first and second conductive grids (38 & 44)
positioned within the housing (14). A plurality of
preferably cross linked polymer non-metallic cores each
having a uniform conductive exterior metallic surface formed
of a high hydrogen absorbing material, such as metallic
hybride forming material, form a bed (35) of conductive
beads (36) closely packed within the housing (14) in
electrical contact with the first grid (38) adjacent the
inlet (54).; An electric power source (15, 16) in the system
(10) is operably connected across the first and second grid
(38 & 44) whereby electrical current flows between the
grids (38 & 44) and within the aqueous media (59)
flowing through the cell.

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**WO9803699**  
**Nuclear Transmuted Elements Having Unnatural
Isotopic Distributions By Electrolysis And Method Of
Production**   
  
**James Patterson / George Miley**  
  
Also published as:  AU4644097  
  
A method for producing low temperature nuclear
transmutations which occur during electrolysis in an aqueous
medium within a cell (12). New elements produced by
transmutation during operation of the cell are both higher
and lower in atomic mass than the original element
undergoing transmutation. Many of the new elements also
exhibit isotopic shifts from natural isotope abundance. The
electrolytic cell (12) includes a non-conductive housing
(14) having an inlet (54) and an outlet (56) and spaced
apart first and second conductive grids (38 and 44)
positioned within the housing (14).; A plurality of
preferably cross-linked polymer non-metallic cores each
having a uniform conductive exterior metallic surface formed
of a high hydrogen absorbing material, such as a metallic
hydride forming material, form a bed (35) of conductive
beads (36) closely packed within the housing (14) in
electrical contact with the first grid (38) adjacent the
inlet (54). An electric power source (15, 16) in the system
(10) is operably connected across the first and second grid
(38 and 44) whereby electrical current flows between the
grids (38 and 44) and within the aqueous medium (59) flowing
through the cell (12) during cell operation.

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**US2003226401**   
**Atomic structure recognition and modification
method and
apparatus**  
  
**H. Letovsky**  
  
Also published as: US2005145031 // US2005155340  
  
The present invention provides methods and apparatus for
determining the precise makeup of atomic and molecular
structures, as well as providing the capability of modifying
said structures. The invention uses induced resonant
frequency wave effects to define and modify the
electromagnetic, electrical, radioactive, atomic weight, and
co-valent bonding characteristics of matter. One embodiment
of the present invention may produce directionally
controllable magnetic fields in gaseous media that interact
with magnetically polarized vehicle surfaces to allow
high-speed, highly energy efficient inter-planetary space
travel. Another embodiment of the invention may neutralize
waste products remaining from nuclear fission power
production. The invention utilizes controlled multi-spectrum
frequency induction to catalyze changes in atomic structures
that may include: focused and dramatically amplified release
of energy relative to natural states of matter; production
of new alloys; transmutation of dangerous organic compounds
into non-toxic media; and controlled polarization of matter.
The benefits of the invention may include highly efficient
interstellar spacecraft propulsion systems, hazardous waste
elimination systems, efficient electricity production, and
health enhancement of biological organisms.

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**EP1202290**   
**Nuclide transmutation device and nuclide
transmutation
method**  
  
**Y. Iwamura  / T. Itoh**  
  
Also published as:  EP1202290 / US2012269309 /
US2012263265 / US2002080903  
  
The present invention produces nuclide transmutation using a
relatively small-scale device. The device (10) that produces
nuclide transmutation comprises a structure body (11) that
is substantially plate shaped and made of palladium (Pd) or
palladium alloy, or another metal that absorbs hydrogen (for
example, Ti) or an alloy thereof, and a material (14) that
undergoes nuclide transmutation laminated on one surface
(11A) among the two surfaces of this structure body (11).;
The one surface (11A) side of the structure body (11), for
example, is a region in which the pressure of the deuterium
is high due to pressure or electrolysis and the like, and
the other surface (11B) side, for example, is a region in
which the pressure of the deuterium is low due to vacuum
exhausting and the like, and thereby, a flow of deuterium in
the structure body (11) is produced, and nuclide
transmutation is carried out by a reaction between the
deuterium and the material (14) that undergoes nuclide
transmutation.

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**WO0231833**   
**Nuclear Transmutational Processes**  
  
**Arie De Geus**  
  
The invention relates to a method of generating energy,
comprising the steps of: a. introducing hydrogen in a
reactor vessel, the vessel comprising a cathode, an anode
and an ionization element, the cathode comprising a primary
and a secondary transmutational element, the transmutational
elements having in their nucleus a number of neutrons which
is larger than the number of protons, and wherein at least
one neutron has a preferred orientation; b. Ionizing at
least a part of the hydrogen with the ionization element to
form a plasma, c. Applying a voltage differential across the
cathode and the anode, causing protons to travel to the
cathode and to induce a transmutation of the transmutational
elements which combine to form an element of higher mass
number than the mass number of said transmutational elements
under the release of energy; and d. collecting heat and/or
on other energy formed in step c. In a preferred embodiment
the primary transmutational element comprises formula (i) or
any combination thereof, whereas the secondary
transmutational element comprises formula (ii) or any
combination thereof.

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**NL1031962**   
**Energy generating process for producing
electricity, comprises electron discharge in flow of
nitrogen or air in order to cause nuclear transmutation of
nitrogen into carbon
monoxide**   
  
**A. de Geus**  
  
A flow of nitrogen or air, or a plasma thereof, through a
reactor (1) is exposed to an electron discharge, resulting
in the nuclear transmutation of gaseous nitrogen into carbon
monoxide, followed by oxidation of the carbon monoxide to
carbon dioxide. A method for generating energy comprises
passing a continuous flow of nitrogen or air, or a plasma
thereof, through an optionally enclosed reactor in which
electron discharge takes place, resulting in the nuclear
transmutation of gaseous nitrogen into carbon monoxide,
followed by oxidation of the carbon monoxide to carbon
dioxide. An INDEPENDENT CLAIM is also included for the
process apparatus, comprising a reactor with a pressure
reducing means (6) and an inlet (7) for providing an
intermittent supply of nitrogen or air; at least one cathode
and at least one anode on the inner side of the reactor
space ends; a means connected to the cathode (4) and anode
(5), used for generating high voltage pulses with a
predetermined waveform and frequency between the cathode and
anode; a casing around the reactor, through which air flows
in order to be heated by the process heat from the reactor;
and optional conduits for recirculating the heat-laden air
back to the casing.

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**WO03025951**  
**Multi-Step, Time Programmed Procedure For The
Transmutation Of Radioactive Wastes And Multi-Region Salt
Melt Apparatus For Carrying Out The
Procedure**   
  
**G. Csom / A.  Aszodi**  
  
Also published as:     HU226177 / HU0103762
/  US2005013397 / RU2004111795 /   JP2005503568  
  
A radiocactive waste containing medium is circulated within
two or more systems (1,2,3) separated from each other
flowtechnically; and the circulated radioactive waste is
exposed to neutron radiations of different energy spectrum
in each system by operating a reactor physically united
entirety of irradiated sections of the said systems as a
nuclear reactor or an accelerator driven subcritical system.
Each system (1,2,3) has a heat exchanger (9,10) and, in
given cases, a circulating pump (10,21) and an expansion
tank (5,16,27). The disclosed apparatus has two or more
reactor regions (1,2,3) separated from each other by
partitions (37,38) and, preferably, arranged coaxially
within a reactor space encircled by a common shell structure
(39). A particle beam (45) produced by a particle
accelerator is preferably directed into the innermost
reactor region (3).

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**WO9735324**  
**Method For Preparing Highly Radioactive
Materials For Transmutation And/Or
Burn-Up**   
  
**C. Fuch s / S. Fourcaudo**  
  
Also published as:  GR3036593 / PT888623 / LU88727 /
JP2000506976 /  ES2159115  
  
The invention concerns a method of preparing highly
radioactive materials for transmutation and/or burn-up by
irradiation in a nuclear plant. The invention proposes that
the materials are first converted into liquid form by
melting or chemical dissolution and a porous carrier
material which is essentially insoluble in the liquefied
materials is impregnated with the liquefied materials and
then heated in such a way that the materials are converted
into the finally required chemical form and density.

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**RU2212072**  
**Method And Device For Transmutation Of
Radioactive Wastes**  
  
**A. V. Levadnyj / K. Rutkovskaja**  
   
 FIELD: nuclear power engineering. SUBSTANCE: proposed
method and device are intended for power generation,
transmutation of radioactive wastes, burnout of weapon
plutonium and actinides. Interaction of neutron beam coming
from neutron generator is effected on lead matrix wherein
nuclear fuel and radioactive wastes are distributed; then
they are decelerated and bred in subcritical thermal core.
Device implementing this method has its central target made
in the form of lead matrix with nuclear fuel and radioactive
wastes distributed therein. EFFECT: enhanced efficiency of
transmutation process.

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**RU2343575**   
**Method Of Long-Living Radionuclides Fixation For
Storage And Transmutation**   
  
**V. Tikhonov  / K. Kapustin**  
  
FIELD: chemistry, waste recycling. ^ SUBSTANCE: invention
relates to field of liquid radioactive wastes recycling.
Long-living radionuclides are isolated from nitric acid
solution of used nuclear fuel (UNF) into solid phase in form
of acetates, oxides and other compounds, which do not
contain elements strongly activated with neutrons.
Radionuclides are imbedded and fixed in carbon matrix.
Carbon matrix is obtained in process of carrying out
reaction of metal acetates with excess of phthalonitryl and
their further pyrolysis. For radionuclides isolated from UNF
in form of oxides or other compounds, carbon matrix is
obtained by their mixing with yttrium acetate, then
synthesis and pyrolysis of yttrium diphthalocyanine are
carried out. Operation of synthesis and pyrolysis of yttrium
diphthalocyanine is carried out in inert atmosphere,
pyrolysis is carried out at T=850-1100 DEG C.; Obtained
carbon matrix does not contain elements strongly activated
with neutrons, which allows using it both for long-term
storage and for transmutation of long-living radionuclides
without any chemical processing and additional operations. ^
EFFECT: obtaining carbon matrix which can be used both for
long-term storage and for transmutation of long-living
radionuclides without any chemical processing and additional
operations.

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**RU2156001**  
**Radioactive Waste Processing Technique**  
  
**B. Taratorin / S. Ivanov**  
  
SUBSTANCE: radioactive wastes are placed in nuclear
explosion zone of weapon plutonium wherein intensive neutron
flux is allowed to pass through them to convert them to
steam that condenses into particles measuring about 10-6 cm.
Neutron flux and heat energy released due to explosion of
weapon plutonium cause transmutation of nuclides in desired
quantities and their separation into long- and short-living
ones in condensed state from steam by centrifuging. Proposed
technique provides for using products of explosion to
produce electrical energy and transuranium elements. EFFECT:
provision for peaceful use of weapon plutonium.

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**CN101325092**   
**Solution stack for burning plutonium and
transmutation of neptunium-237 or americium-241**  
  
**Wu Yinghua / W.  Lianjie**  
  
The invention discloses a solution reactor used for the
plutonium combustion and the neptunium-237 or the
americium-241 transmutation. The solution reactor adopts
plutonium or plutonium and americium in the spent fuel of
the nuclear power plant as the fuel, and adopts
neptunium-237 or americium-241 as the target. By adopting
the solution reactor, the minor actinides which have long
half life and high toxicity and can not be stored for a long
time, such as the neptunium-237 or the americium-241, can be
changed into nuclides with short half life and low toxicity
through transmutation. Because the solution reactor adopts
the spent fuel and can generate electricity at the low
temperature, the cost-effectiveness and the security are
high; the neutron provided by the plutonium combustion can
extract plutonium-238 from the neptunium-237 solution target
as the isotope battery, thereby the inexpensive energy is
provided; the americium-242m extracted from the
americium-241 solution target can be widely applied to the
aerospace industry and the medical industry

---

**US2008240330**  
**Compact Device for Dual Transmutation for
Isotope Production Permitting Production of Positron
Emitters, Beta Emitters and Alpha Emitters Using Energetic
Electrons**   
  
**Charles Holden**  
  
A method and apparatus for directing high energy electrons
to a converter material that emits gamma rays, which, in
turn interact directly with parent isotopes to produce
unstable, short-lived medical isotopes and product isotopes
by the gamma, n reaction, or which interact with high-z
materials to produce neutrons that then produce valuable
isotopes by neutron capture in parent isotopes.

---

**NL1033078**   
**Energy generating process, by applying voltage
between cathode comprising transmutation elements and
anode in reactor vessel containing plasma**  
        
Arie de Geus  
  
The process comprises the following steps: (A) adding
hydrogen to a reactor vessel (6) containing a cathode (8),
anode (9) and optionally an ionization element; the cathode
comprises a primary and secondary transmutation element, the
cores of which contain more neutrons than protons; the
primary element contains a neutron with a preferable
orientation; (B) ionizing at least some of the hydrogen to
form a plasma; (C) applying a voltage difference with a
given time character between the cathode and anode, causing
a flow of protons towards the cathode, to which they become
temporarily bonded; the transmutation elements next to the
cathode surface and in the resulting plasma vortex fuse to
form an element with a higher mass number and a second
element or molecule with a lower mass number; and (D)
collecting the radiation, which can be converted directly
into electricity or heat.

---

**US2005155340**  
**Method and apparatus for the transmutation of
nuclear waste with tandem production of tritium**  
  
El-Sharawy  / El-Badawy  
  
Also published as: US2005145031 / AU2001297883   
  
The transmutation of radioactive material using a hybrid
transmutation reactor is disclosed wherein a kinetic proton
source is used to collisionally induce the transmutation of
radioactive material with the generation of thermal neutrons
as a byproduct. Additionally, a system and method for the
production of Tritium utilizing the thermal neutrons
generated in the transmutation process is further described.
The present invention offers advantages and improvements
over existing nuclear reactor technologies in that nuclear
waste may be rendered inert, or otherwise at least partially
deactivated and/or made less dangerous, with the
substantially simultaneous production of energy and/or
Tritium as a byproduct of the transmutation process.

---

**US2009135981**  
**Element Transmutation Method And Energy
Generation Method**  
  
**Norio Yabuuchi**  
  
Also published as:  JP2009128300  
  
PROBLEM TO BE SOLVED: To achieve a reliable method to output
energy using nucleus condensation. ; SOLUTION: Deuterium
nuclei are coordinated at vertical angle positions of each
face constituting a regular hexahedron, inside a metallic
crystal. Electrons are coordinated to the other vertical
angle positions. By Coulomb attraction acting between four
protons and four electrons, four deuterium nuclei are fused
to transmute into two helium atoms

---

**US6442226**   
**Accelerator-driven transmutation of spent fuel
elements**  
  
**Venneri, et al.**  
  
An apparatus and method is described for transmuting higher
actinides, plutonium and selected fission products in a
liquid-fuel subcritical assembly. Uranium may also be
enriched, thereby providing new fuel for use in conventional
nuclear power plants. An accelerator provides the additional
neutrons required to perform the processes. The size of the
accelerator needed to complete fuel cycle closure depends on
the neutron efficiency of the supported reactors and on the
neutron spectrum of the actinide transmutation apparatus.
Treatment of spent fuel from light water reactors (LWRs)
using uranium-based fuel will require the largest
accelerator power, whereas neutron-efficient high
temperature gas reactors (HTGRs) or CANDU reactors will
require the smallest accelerator power, especially if
thorium is introduced into the newly generated fuel
according to the teachings of the present invention. Fast
spectrum actinide transmutation apparatus (based on
liquid-metal fuel) will take full advantage of the
accelerator-produced source neutrons and provide maximum
utilization of the actinide-generated fission neutrons.
However, near-thermal transmutation apparatus will require
lower standing inventories of plutonium and higher
actinides. Uranium, presently the largest volume constituent
in nuclear waste, is fully utilized and not discharged as
waste. Since no plutonium, higher actinides or fission
products are present in the reconstituted fuel elements, the
present processes can be used repeatedly. Since the
performance of the existing reactors is not changed, full
utilization of both thorium and uranium resources is
achieved.

---

**US6738446**  
**System and method for radioactive waste
destruction**   
  
**Mike Venneri / Francesco Baxter**  
  
Also published as: WO2004040588 / CN101061552  
  
A method for transmuting spent fuel from a nuclear reactor
includes the step of separating the waste into components
including a driver fuel component and a transmutation fuel
component. The driver fuel, which includes fissile materials
such as Plutonium<239>, is used to initiate a
critical, fission reaction in a reactor. The transmutation
fuel, which includes non-fissile transuranic isotopes, is
transmuted by thermal neutrons generated during fission of
the driver fuel. The system is designed to promote fission
of the driver fuel and reduce neutron capture by the driver
fuel. Reacted driver fuel is separated into transuranics and
fission products using a dry cleanup process and the
resulting transuranics are mixed with transmutation fuel and
re-introduced into the reactor.; Transmutation fuel from the
reactor is introduced into a second reactor for further
transmutation by neutrons generated using a proton beam and
spallation target.

---

**JP2007322202**   
**Method, Device And Program For Predicting
Nuclear Reaction In Flocculation System, And Method For
Detecting Substance After Nuclide
Transmutation**   
  
**Ito Takehiko / Iwamura Yasuhiro**  
  
PROBLEM TO BE SOLVED: To provide a method for predicting
nuclear reaction in a flocculation system which enables
high-accuracy prediction of the nuclear reaction. ;
SOLUTION: In the method for predicting the nuclear reaction
in the flocculation system, where a substance which is
subjected to nuclide transmutation is placed in contact with
a structure in the flocculation system and deuterium is made
to flow into it to induce nuclear reaction in the substance
which is subjected to nuclide transmutation; a substance
where 2n (n is a natural number) is added to both the atomic
number and the mass number, respectively of the substance to
which nuclide transmutation is given is predicted as being
the substance to be generated after the nuclide
transmutation.

---

**WO2006005813**   
**Method And Device For Transmutation Of Nucleons
Free Of Prior Or Permanent
Plasma**  
  
**G. Vitrac**  
  
The invention concerns a method and a device for
transmutation of nucleons free of prior or permanent plasma
to provide particles whereof the kinetic energy is
quantified for resonance of the active section for
specialized application. The exact distribution results from
vector compositions of quanta generated by structural
piezoelectric actuators and spin inducers. The fusion is
then obtained by activation ad minima tunnel effect. The
economy and reliability of the system are linked to the
programming of quantum models representative of discrete
cycles, and the minimized supply of reagents with
stage-recycling possibilities, and annihilations, while
promoting the option of low level radiation. Various fields
of application concern said inventive mini-reactor such as
radiochemistry, medical imaging and non-destructive
controls, selection and treatments of waste.

---

**US2004047443**  
 **Electron capture by magnetic resonance**  
  
 **E. Bondoc**  
  
The process of capturing electron by subjecting proton to
magnetic resonance until its magnetic moment is in opposite
direction relative to the electron's magnetic moment. As
soon as the particles' magnetic moments are opposite in
direction, spinlocking technique is applied for a period of
time to induce transmutation of the particles and the
consequent reactions of the product with an adjacent
particle or a group of particles and the release of energy.

---

**US2007297554**   
**Method And System For Production Of
Radioisotopes, And Radioisotopes Produced
Thereby**   
  
**E. Lavie / I. Silverman**  
  
Also published as: WO2006035424 / EP1807844 / EP1807844 /
AT468589  
  
A system and method for the production of radioisotopes by
the transmutation of target isotopic material bombarded by a
continuous wave particle beam. An ion source generates a
continuous wave ion beam, irradiating an isotope target,
which is cooled by transferring heat away from the target at
heat fluxes of at least about 1 kW/cm<2>.

---

**US2003016774**  
**Method and apparatus for stimulated beta decays**  
  
**R. Santilli**  
  
Method for the synthesis of neutrons from protons and
electrons comprising apparatus for said protons and
electrons to have a threshold relative energy of about 0.80
MeV, for said protons and electrons to be in anti-parallel
coupling, and for forcing said protons and electrons in
anti-parallel coupling to be at a mutual distance
essentially of one Fermi. Another embodiment includes a
method for the stimulated decay of a peripheral neutron in a
nucleus. Another embodiment includes apparatus for the
stimulated beta decay of a natural isotope into another
natural isotope, the latter having the same number of
nucleons of the former and one additional proton, wherein
the conservation of total energy, angular momentum and
parity are satisfied. Another embodiment includes apparatus
for the stimulated beta decay of radioactive waste.

---

**US8373087**  
**A PLASMA TORCH FOR USE IN A WASTE PROCESSING
CHAMBER**  
  
Also published as: WO2006114793 / KR20080005986 /
JP2008539061   
  
The invention is a plasma torch for insertion through an
opening in the wall of a waste processing chamber. The
plasma torch of the invention is characterized by comprising
a coaxial sleeve having an upper end and a lower end. The
sleeve surrounds at least the portion of the outer surface
of the torch that is located in the opening, thereby forming
an insulating chamber between the outer surface if the torch
and the inner surface of the sleeve. At least a portion of
the portion of the coaxial sleeve that surrounds at least
the portion of the outer surface of the torch that is
located in the opening in the wall of the processing chamber
is porous or permeable to a heat exchanging fluid. The torch
comprises an inlet for introducing the heat exchanging fluid
into the insulating chamber. When the plasma torch is
inserted through the opening, a gap exists between the
processing chamber wall and the coaxial sleeve. Thus the
coaxial sleeve and the insulating chamber shield the outer
surface of the plasma torch from a significant amount of the
heat that radiates from the processing chamber wall and from
inside the processing chamber and the heat exchanging fluid
that flows through the inlet exits the insulating chamber
into the processing chamber.

---

**US8090072**  
**Neutron-driven element transmuter**  
  
**Carlo Rubbia**  
   
Also published as: WO9859347 / US7796720 / SK166999 /
SK286044  
   
A material is exposed to a neutron flux by distributing it
in a neutron-diffusing medium surrounding a neutron source.
The diffusing medium is transparent to neutrons and so
arranged that neutron scattering substantially enhances the
neutron flux to which the material is exposed. Such enhanced
neutron exposure may be used to produce useful
radioisotopes, in particular for medical applications, from
the transmutation of readily-available isotopes included in
the exposed material. It may also be used to efficiently
transmute long-lived radioactive wastes, such as those
recovered from spent nuclear fuel. The use of heavy
elements, such as lead and/or bismuth, as the diffusing
medium is particularly of interest, since it results in a
slowly decreasing scan through the neutron energy spectrum,
thereby permitting very efficient resonant neutron capture
in the exposed material.

---

**JP2005062025**   
**Method For Increasing Nuclear Transmutation
Quantity From Nuclear Transmutation Device And Nuclear
Transmutation Device**  
  
**M. Sakano / T. Ito**  
  
To provide a method for increasing a nuclide quantity which
enables transmutation from a nuclear transmutation device in
the first nuclear transmutation process, and a nuclear
transmutation device. ; SOLUTION: With this method, a
nuclear transmutation quantity from a nuclear transmutation
device is increased by a process for applying electrolysis
process or plasma treatment to a surface of a structure
including a hydrogen occlusion metal, and adding a material
causing nuclear transmutation to the surface

---

**WO2008041254**  
**APPARATUS AND PROCESS FOR THE PRODUCTION OF
NEUTRONS BY MEANS OF ULTRASOUNDS AND THE CAVITATION OF
SUBSTANCES**  
  
**Fabio CARDONE**  
  
The invention relates to an apparatus and a process for the
production of neutrons in doses which are not dangerous for
living beings, starting from stable elements by means of
insonation or sonication using an electromechanical
transducer, called a sonotrode-cavitator, characterized in
that said electromechanical transducer comprises a stack of
piezoelectric elements mechanically connected to a sonotrode
of such a size as to operate at its own resonance frequency
as a function of the electrical activation energy applied to
said piezoelectric elements. The process is conducted in the
liquid phase, preferably in the presence of iron ions at
atmospheric pressure in an open environment to make the
bubbles naturally present in the liquid phase implode.

---

**WO2008041255**  
**PROCESS AND PLANT FOR THE PRODUCTION OF
ENDOTHERMIC AND EXOTHERMIC PIEZONUCLEAR REACTIONS BY MEANS
OF ULTRASOUNDS AND THE CAVITATION OF SUBSTANCES**  
  
**Fabio CARDONE**  
  
Also published as:  ITRM20060522  
  
The invention relates to a process and plant for the
production of endothermic and exothermic piezonuclear
reactions by means of ultrasounds and the cavitation of
substances. The plant comprises in sequence a storage tank
for the working liquid containing an active medium in
solution and/or in suspension, said storage tank being
connected up to a cavitation chamber in which the
piezonuclear reactions take place. In the case of exothermic
reactions, there is production of vapour under high
pressure, which is then conveyed to a turbine for the
production of mechanical energy or electrical energy by
means of an alternator or equivalent; the process is
accompanied by the secondary phenomenon of production of
material different from that making up the working liquid.
In the case of endothermic reactions, there is consumption
of electrical energy for the generation of piezonuclear
reactions that produce substances regarded as useful
starting from the working liquid available.

---

**WO2008041253**  
**APPARATUS AND PROCESS FOR THE QUENCHING OF THE
RADIOACTIVITY OF RADIOACTIVE MATERIALS BY MEANS OF
PIEZONUCLEAR REACTIONS INDUCED BY ULTRASOUNDS AND
CAVITATION**  
  
**Fabio CARDONE**  
  
The invention relates to an apparatus and a process for
reducing the radioactivity of natural and/or artificial
elements through piezonuclear reactions generated by means
of insonation or sonication using an electromechanical
transducer. The apparatus is characterised in that said
electromechanical transducer comprises a stack of
piezoelectric elements mechanically connected to a sonotrode
of such a size as to operate at its own resonance frequency
as a function of the electrical activation energy applied to
said piezoelectric elements, to obtain the cavitation of the
bubbles present in the liquid in which the radioactive
substances are to be placed.

---

**US6233299**   
 **Assembly for transmutation of a long-lived
radioactive material**  
  
 **Wakabayashi**  
  
Abstract -- A new transmutation assembly permits an
efficient transmutation of a long-lived radioactive material
(long-lived FP nuclides such as technetium-99 or iodine-129)
which was produced in the nuclear reactor. Wire-type members
of a long-lived radioactive material comprised of metals,
alloys or compounds including long-lived FP nuclides are
surrounded by a moderator material and installed in cladding
tubes to form FP pins. The FP pins, and nothing else, are
housed in a wrapper tube to form a transmutation assembly.
The wire-type members can be replaced by thin ring-type
members. The transmutation assemblies can be selectively and
at least partly loaded into a core region, a blanket region
or a shield region of a reactor core in a fast reactor. From
a viewpoint of reducing the influence on the reactor core
characteristics, it is optimal to load the transmutation
assemblies into the blanket region.

---

**US6233298**   
 **Apparatus for transmutation of nuclear reactor
waste**  
  
 **Bowman**  
  
A subcritical reactor-like apparatus for treating nuclear
wastes, the apparatus comprising a vessel having a shell and
an internal volume, the internal volume housing graphite.
The apparatus having means for introducing a fluid medium
comprising molten salts and plutonium and minor actinide
waste and/or fission products. The apparatus also having
means for introducing neutrons into the internal volume
wherein absorption of the neutrons after thermalization
forms a processed fluid medium through fission chain events
averaging approximately 10 fission events to approximately
100 fission events. The apparatus having additional means
for removing the processed fluid medium from the internal
volume. The processed fluid medium typically has no
usefulness for production of nuclear weapons.

---

**US5160696**   
 **Apparatus for nuclear transmutation and power
production using an intense accelerator-generated thermal
neutron flux**  
  
 **Bowman**  
  
Apparatus for nuclear transmutation and power production
using an intense accelerator-generated thermal neutron flux.
High thermal neutron fluxes generated from the action of a
high power proton accelerator on a spallation target allows
the efficient burn-up of higher actinide nuclear waste by a
two-step process. Additionally, rapid burn-up of fission
product waste for nuclides having small thermal neutron
cross sections, and the practicality of small material
inventories while achieving significant throughput derive
from employment of such high fluxes. Several nuclear
technology problems are addressed including 1. nuclear
energy production without a waste stream requiring storage
on a geological timescale, 2. the burn-up of defense and
commercial nuclear waste, and 3. the production of defense
nuclear material. The apparatus includes an accelerator, a
target for neutron production surrounded by a blanket region
for transmutation, a turbine for electric power production,
and a chemical processing facility. In all applications, the
accelerator power may be generated internally from fission
and the waste produced thereby is transmuted internally so
that waste management might not be required beyond the human
lifespan.

---

**US 5848110 /** **US5764715**   
 **Method and apparatus for transmutation of
atomic nuclei**  
  
 **Maenchen, et al.**  
  
The present invention addresses the problems outlined above.
An accelerator based on a combination of a high repetition
rate high energy pulsed power supply (RHEPP) and a
magnetically-injected anode plasma (MAP) source diode is
used to provide pulsed particle beams having intermediate
energy (0.2-20 MeV) and average power levels of hundreds of
kilowatts to megawatts. This will increase the rate of
isotopic production by 2-3 orders of magnitude over
processes based on conventional accelerators. Any gaseous
ion can be accelerated with this technology (proton,
deuteron, and helium beams are of special interest). This
capability can be applied to transmute target nuclei
selectively into desired isotopes. RHEPP/MAP accelerators
are also extremely power efficient and relatively small in
size, making application of small units practical in, for
example, major local or regional medical facilities.
Finally, the use of relatively low beam particle energies
reduces or eliminates the problem of undesired products and
the subsequent generation of radioactive waste. Although the
invention is being discussed in terms of embodiment via the
RHEPP/MAP system, any pulsed ion beam generator having
sufficient ion kinetic energy and total average beam current
can be used in the same manner.

---

**US 4961880**  
**Electrostatic Voltage Excitation Process and
Apparatus**  
  
**William A. Barker**  
  
Accelerated decay of radioactive materials is used for power
production. In the method of this invention an
alpha-emitting radioactive material is placed in a region.
The region is selected so that when a negative potential is
applied to the region, enhanced alpha decay of the
radioactive material results. The energy of the alpha decay
particles is captured and converted to thermal energy.

---

**US
Patent 5076971**  
 **Method for Enhancing Alpha
Decay in Radioactive Materials**

 

**William
Barker**

Apparatus and method for decontaminating
radioactive materials by stimulating the atomic system of
radioactive materials. The stimulus is kept applied to the
radioactive materials for a predetermined time. In this way,
the rate of decay of the radioactivity of the materials is
greatly accelerated and the materials are thereby
decontaminated at a rate much faster than normal. The
stimulus can be applied to the radioactive materials placing
them within the sphere or terminal of a Van de Graaff
generator and allowing them to be subjected to the
electrical potential of the generator, such as in the range
of 50 kilovolts to 500 kilovolts, for at least a period of
30 minutes or more.

---

**US2003138068**  
**Method for
Transmutation of Long-Living Radioactive
Isotopes into Short-Living or Stable Ones**

**V.S.
Buttsev, et al.**

Also published as: EP1274099 // WO0173474 / RU2169405

Nuclear physics; decontamination of
radioactive wastes and the like from long-living radioactive
isotopes. Substance: transmutation of long-living
radioactive isotopes into short-living or stable ones is
conducted under the action of electromagnetic radiation. In
the process, highly ionized atoms with energy- resolved hole
of accelerated beta-decay are produced from atoms of
long-living radioactive isotope and held in ionized state
until transmutation of mother nuclei to daughter
short-living or stable ones takes place. With coefficient of
operating time k preset for daughter nuclei, atoms of
long-living radioactive isotope are held in highly ionized
state for at least time beta, where beta is lifetime of
mother nuclei under accelerated beta-decay conditions.
Electromagnetic radiation may be effected by beams of
accelerated charged particles (electrons, protons, or ions)
or by photon flux. Radiation by charged-particle beam may be
combined with photonflux radiation. Effect:  enhanced
transmutation efficiency dispensing with nuclear reactions
of collision character and avoiding formation of
by-products.

---

**US
Patent Appln. # 2002186805**  
 **Accelerated Radioactivity
Reduction**

 

**Sidney
Soloway**

A method for reducing radioactivity in a
radioactive sample is disclosed, comprising contacting said
sample with a beam of photons, said beam having an energy
level sufficient to cause said radioactive sample to emit
particles including photons in an amount sufficient to
accelerate a reduction in radioactivity of said sample. Also
disclosed is a method of increasing radioactive decay in a
radioactive isotope comprising the steps of: determining a
beam of an effective energy and effective flux of photons to
increase radioactive decay in the radioactive isotope;
applying the beam to the radioactive isotope; and
maintaining the beam for an amount of time effective to
increase the radioactivity of the radioactive isotope.

---

**US
Patent Appln.  20040238366**  
 **Method and System with
Apparatus for Acceleration of Activity Decrease
and Radioactive Material Deactivation**

 

**Vladimirovich,
Kinderevich, et al.**

Radioactive material can be processed by an
apparatus that includes at least a cylindrical outer shell
electrode, an inner electrode, and a plurality of
prism-shaped ferromagnetic elements positioned between the
outer and inner electrodes. The prism-shaped ferromagnetic
elements are positioned around the inner circumference of
the metal cylinder. The inner electrode component is located
within the metal cylinder and is configured to cover the
inwardly-pointing portions of the prism-shaped ferromagnetic
elements. Radioactive material in a container is placed into
the apparatus, and an AC voltage excitation signal is
applied to the electrodes of the apparatus during treatment
of the material. The frequency of the excitation signal is
selected according to the frequency of structurization or
the frequency of destructurization of the ferromagnetic
material. The process can be monitored and controlled with
the use of alpha, beta, and gamma radiation intensity
measuring instruments.

---